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Yamane, Yuichi; Amano, Yuki; Tashiro, Shinsuke; Abe, Hitoshi; Uchiyama, Gunzo; Yoshida, Kazuo; Ishikawa, Jun
Journal of Nuclear Science and Technology, 53(6), p.783 - 789, 2016/06
Times Cited Count:6 Percentile:43.12(Nuclear Science & Technology)The release behavior of radioactive materials from high active liquid waste (HALW) has been experimentally investigated under boiling accident conditions. In the experiments using HALW obtained through laboratory scale reprocessing, release ratio was measured for the FP nuclides such as Ru, Tc, Cs, Sr, Nd, Y, Mo, Rh and actinides such as Cm, Am. As a result, the release ratio was 0.20 for Ru and 1 for the FP and Ac nuclides. Ru was released into the gas phase in the form of both mist and gas. For its released amount, weak dependency was found to the initial concentration in the test solution. The release ratio decreased with the initial concentration. For other FP nuclides and actinides as non-volatile, released into the gas phase in the form of mist, the released amount increased with the initial concentration. The release ratio of Ru and NOx concentration increased with temperature of the test solutions. They were released almost at the same temperature between 200 and 300C. Size distribution of the mist and other particle was measured.
Oigawa, Hiroyuki; Yokoo, Takeshi*; Nishihara, Kenji; Morita, Yasuji; Ikeda, Takao*; Takaki, Naoyuki*
Proceedings of International Conference on Nuclear Energy System for Future Generation and Global Sustainability (GLOBAL 2005) (CD-ROM), 6 Pages, 2005/10
The benefit of implementing Partitioning and Transmutation (P&T) of high-level wastes was parametrically surveyed. The possible reduction of the geological repository area was estimated. By recycling minor actinides (MA), the repository area required for unit spent fuel was reduced significantly in the case of MOX-LWR. This effect was caused by removal of Am which is a long-term heat source. By partitioning the fission products, in addition to MA recycling, further 70-80% reduction from the MA-recovery case can be expected for both UO and MOX. This significant reduction was independent of the cooling time before the partitioning process.
Morita, Yasuji; Kubota, Masumitsu*
JAERI-Review 2005-041, 35 Pages, 2005/09
Research and development on Partitioning in JAERI are reviewed in the present report from the beginning to the development of the 4-Group Partitioning Process and its test with real high-level liquid waste (HLLW). In the 3-Group Partitioning Process established in around 1980, elements in HLLW are separated into 3 groups of transuranium element group, Sr-Cs group and the other element group. The 4-Group Partitioning Process subsequently developed contains the separation of Tc-platinum group metals additionally. The process was tested to demonstrate its performance with real concentrated HLLW. Until then, various separation methods for various elements were studied and selection and optimization of the separation methods were carried out to establish the process. Review of the experience, findings and results is very important and valuable for future study on partitioning. The present report is prepared from this point of view.
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Nihon Genshiryoku Gakkai-Shi, 16(9), p.478 - 485, 1974/09
no abstracts in English
Funtai Oyobi Fummatsu Yakin, 8(4), p.137 - 144, 1961/00
no abstracts in English